Evolution of the Luminescence Properties of Single CsPbBr3 Perovskite Nanocrystals During Photodegradation

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Abstract

The evolution of the luminescence blinking of single CsPbBr3 perovskite nanocrystals with a characteristic size of ~25 nm during photodegradation has been experimentally investigated. It has been demonstrated that the blue shift of the luminescence peak and a decrease in the average luminescence intensity are accompanied by the increasing role of nonradiative Auger processes underlying the charging mechanism of blinking. A method based on the analysis of photon antibunching g2(0) and exciton and biexciton recombination rates is used to determine the blinking mechanism. The data obtained have made it possible to reveal a transition from the trapping to charging blinking mechanism with a change in the sizes of a CsPbBr3 single nanocrystal.

About the authors

V. A. Baitova

HSE University

Email: eremchev@isan.troitsk.ru
105066, Moscow, Russia

M. A. Knyazeva

HSE University;Troitsk Separate Branch, Lebedev Physical Institute, Russian Academy of Sciences

Email: eremchev@isan.troitsk.ru
105066, Moscow, Russia;108840, Troitsk, Moscow, Russia

I. A. Mukanov

Institute of Spectroscopy, Russian Academy of Sciences;Moscow Institute of Physics and Technology (National Research University)

Email: eremchev@isan.troitsk.ru
108840, Moscow, Russia;141701, Dolgoprudnyi, Moscow region, Russia

A. O. Tarasevich

Troitsk Separate Branch, Lebedev Physical Institute, Russian Academy of Sciences

Email: eremchev@isan.troitsk.ru
108840, Troitsk, Moscow, Russia

A. V. Naumov

Troitsk Separate Branch, Lebedev Physical Institute, Russian Academy of Sciences;Institute of Spectroscopy, Russian Academy of Sciences;Moscow Pedagogical State University

Email: eremchev@isan.troitsk.ru
108840, Troitsk, Moscow, Russia;108840, Moscow, Russia;119435, Moscow, Russia

A. G. Son

Moscow Institute of Physics and Technology (National Research University);Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences

Email: eremchev@isan.troitsk.ru
141701, Dolgoprudnyi, Moscow region, Russia;119991, Moscow, Russia

S. A. Kozyukhin

Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences;Faculty of Chemistry, Tomsk State University

Email: eremchev@isan.troitsk.ru
119991, Moscow, Russia;634050, Tomsk, Russia

I. Yu. Eremchev

Institute of Spectroscopy, Russian Academy of Sciences

Author for correspondence.
Email: eremchev@isan.troitsk.ru
108840, Moscow, Russia

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